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The electroreduction of carbon dioxide (CO2) toward high‐value fuels can reduce the carbon footprint and store intermittent renewable energy. The iodide‐ion‐assisted synthesis of porous copper (P‐Cu) microspheres with a moderate coordination number of 7.7, which is beneficial for the selective electroreduction of CO2 into multicarbon (C2+) chemicals is reported. P‐Cu delivers a C2+ Faradaic efficiency...
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