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The coordination environment is crucial for the activity of an electrocatalyst, which defines the interaction between the central and adjacent atoms. In traditional 2D MX2 (M = Mo, W, etc., X = S, Se), M is usually coordinated with 6 X atoms in either trigonal prismatic (2H) or octahedral (1T) polyhedrons. With such a coordination configuration, only the edge X sites exhibit activity for hydrogen...
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