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Gel polymer electrolytes (GPEs) incorporate both the high ionic conductivity of organic liquid electrolyte and the high safety performance of all‐solid‐state electrolytes (ASSEs), greatly improving the electrochemical performance of solid polymer electrolytes (SPEs). However, the practical application of GPEs is still limited by inferior interface compatibility, lithium dendrites, etc. Herein, we...
All‐solid electrolyte instead of frequently‐used inflammable electrolyte can enhance the security and energy density of batteries effectively. However, the low ionic conductivity lead to increased lithium dendrites and increased resistance of the cell at 30 °C. In this work, non‐toxic and low‐cost hydroxypropyl methylcellulose (HPMC) was introduced simultaneously with non‐polluting hectorite (Ht)...
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