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This study deals with a reinvestigation on the maximum oxidation state of gold. Density functional calculations are performed on geometries and stabilities of AuCln species for n = 1–6 in their neutral and anionic states. The calculations clearly reveal that the maximum oxidation state of Au is limited to +5. The high adiabatic electron affinities of AuCln (n ≥ 2), as compared to Cl, suggest their...
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