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The regeneration of ruthenium(II) dyes by cobalt redox mediator in dye-sensitized solar cells (DSSCs) has been investigated using density functional theory combined with the Marcus theory of electron transfer. Our results show that the regeneration reaction rates gradually increase with the growth of the dye protonation degree. By comparing the natures of protonated and deprotonated states, we reveal...
The regeneration processes of triphenylamine (TPA)-based dyes with cobalt redox mediator in dye-sensitized solar cells (DSSCs) have been investigated using density functional theory combined with the Marcus theory of electron transfer. Our results show that with the extension or rigidification of the oligothiophene conjugation linker the absorption spectra of TPA dyes exhibit observable red-shift...
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