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The epitaxial deposition of an oxide semiconductor ZnO thin film was demonstrated on a Pt(111)/sapphire(0001) cathode by local pH control in the vicinity of the cathode. The local pH near the cathode was increased by the selective reduction of NO 3− ions, resulting in the deposition of a ZnO thin film only on the cathode surface by hydrolysis. The pH distribution near the cathode during...
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