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Photoinduced processes in thiouracil derivatives have lately attracted considerable attention due to their suitability for innovative biological and pharmacological applications. Here, sub‐20 fs broadband transient absorption spectroscopy in the near‐UV are combined with CASPT2/MM decay path calculations to unravel the excited‐state decay channels of water solvated 2‐thio and 2,4‐dithiouracil. These...
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