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Sodium superionic conductor (NASICON)‐type Na3V2(PO4)3 has attracted considerable interest owing to its stable three‐dimensional framework and high operating voltage; however, it suffers from a low‐energy density due to the poor intrinsic electronic conductivity and limited redox couples. Herein, the partial substitution of Mn3+ for V3+ in Na3V2(PO4)3 is proposed to activate V4+/V5+ redox couple for...
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