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Rational and efficient conversion of methane to more useful higher hydrocarbons is one of the most important topics of natural gas utilization. Although methane activation and its conversion to valuable compounds attract an increasing attention, methane conversion is often made in indirect way through the very energy-consuming step for syngas production from steam reforming of methane. Some promising...
HSAPO-34 molecular sieve was employed in chloromethane conversion and showed high performance in activity and selectivity in production of light olefins. Our detailed IR investigation allowed the identification of the active sites and the adsorbed species and demonstrated that the conversion started from 350°C with alkoxy group as the intermediate. The fixed-bed catalytic testing evidenced that in...
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