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This paper reports on direct dimethyl ether synthesis from syngas on hybrid bifunctional copper–zeolite catalysts. Both laboratory synthesized and commercial zeolites were used in this work. The catalyst performance is evaluated under pressure in a continuous fixed bed milli-reactor. The relationships between zeolite particle sizes, acidity and catalytic performance of the hybrid catalysts in dimethyl...
Direct synthesis of dimethyl ether (DME) from syngas was investigated on a series of hybrid Cu–ZnO–Al2O3/ZSM-5 catalysts prepared by kneading. It was found that the initial performance of the catalysts was a function of both zeolite crystallite sizes and Si/Al ratio. The activity of the hybrid catalysts gradually decreased with time on stream because of simultaneous copper sintering, copper oxidation...
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