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Single‐atom catalysts (SACs) aim at bridging the gap between homogeneous and heterogeneous catalysis. The challenge is the development of materials with ligands enabling coordination of metal atoms in different valence states, and preventing leaching or nanoparticle formation. Graphene functionalized with nitrile groups (cyanographene) is herein employed for the robust coordination of Cu(II) ions,...
Metal–metal cooperation in a solid‐state mixed‐valence single‐atom catalyst, boosts yield and selectivity in oxidative amine coupling, with uncompromised reusability, as shown by Manoj B. Gawande, Paolo Fornasiero, Radek Zbořil, and co‐workers in article number 1900323. The catalyst, stemming from the chemical entrapment and partial reduction of Cu(II) ions on cyanographene, lays the ground for the...
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