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The stable ionic PdII complexes 1A–4A were synthesized through the complexation of PdCl2(MeCN)2 with the phosphane‐functionalized ionic liquids (FILs) 1–4 with π‐acceptor character. Single‐crystal X‐ray diffraction analyses showed that 1A–4A were all composed of PdII‐centred square‐planar cations and triflate (OTf–, CF3SO3–) counteranions. The complex cations in 1A–3A possessed structural similarity...
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