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The application of high‐performance lithium‐sulfur (Li‐S) batteries is severely influenced by the “shuttle effect” of polysulfides and the volume change of sulfur cathode. Herein, two different polymeric binders SOT‐A and SOT‐C with three‐dimensional network structure containing polar groups (sulfhydryl groups, amide groups and amino groups) are synthesized by the nucleophilic ring‐opening polymerization...
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