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A unique metal addition to the edge of a triangular palladium sandwich cluster is reported. While the edge coordination sites of a parallel sandwich complex are narrow because of two sterically encumbering π‐ligands, association of an additional metal atom to a metal sheet gives a wider coordination site. It was proved that the additional metal atom plays a crucial role in binding of cyclopentadienyl...
The backside‐ligand modulation strategy to enhance the substrate binding property of Pd clusters is reported. The benzene or naphthalene binding ability of Pd3 or Pd4 clusters is enhanced significantly by the backside cyclooctatetraene ligand, leading to the formation of the first solution‐stable benzene‐ or naphthalene Pd clusters. The present results imply that the ligand design of the metal clusters,...
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