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Unrevealed aspects of the photoinduced phase transition are discussed with a special emphasis placed on domains and domain boundaries. The CN− vibration spectroscopy, which is sensitive to the phase changes and boundaries, is applied to photomagnetic phase transition material, RbMn[Fe(CN)6]. From time‐resolved IR measurements for photoinduced low temperature to high temperature phase transition, the...
Structural transformation effect on a photoinduced (PI) charge‐transfer process leading to a phase transition in RbMn[Fe(CN)6], which exhibits a magnetic phase transition with a hysteresis loop between 230 and 300 K, has been investigated by Raman spectroscopy. The valence states of the transition metal ions and the lattice symmetry are reflected in the vibrational frequency of the adjacent CN ions...
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