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An exploratory study on novel silylethynylated N‐heteropentacenes, which have their N atoms on the terminal rings of the pentacene backbone, is reported. This study leads to both p‐ and n‐channel organic thin‐film transistors with high field‐effect mobility and also reveals that the position of the N atoms plays an important role in tuning the structures and properties of organic semiconductors based...
An exploratory study on a group of silylethynylated N‐heteropentacenes as soluble and stable organic semiconductors is presented. An interesting finding is that a silylethynylated N‐heteropentacene can function as a p‐type, n‐type, or ambipolar organic semiconductor depending on the structure of its π‐backbone. The tetraazapentacene derivative is one of the best performing n‐type organic semiconductors...
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