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A series of poly(aryl ether) dendrons with a monopyrrolo‐tetrathiafulvalene unit linked through an acyl hydrazone linkage were designed and synthesized as low molecular mass organogelators (LMOGs). Two of the dendrons could gelate the aromatic solvents and some solvent mixtures, but the others could not gel all solvents tested except for n‐pentanol. A subtle change on the molecular structure produces...
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