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Nonlinear coherent Raman scattering with ultra-short pulse lasers has opened up new opportunities for nonintrusive three-dimensional label-free chemical sensing [1]. A single ultrashort pulse laser, combined to a pulse shaper or a Michelson interferometer (for a review, see [2]), allows for multiplex measurements. However, measuring a broad spectral bandwidth spectrum at high resolution within a very...
Ultra-rapid coherent anti-Stokes Raman spectroscopy with two laser frequency combs is demonstrated. Hyperspectral images are acquired over a spectral bandwidth of 1200 cm−1 with a resolution of 10 cm−1 at a rate of 50 pixels/s.
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