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Solid polymer electrolytes (SPEs) play a pivotal role in advancing electrochemical devices, such as proton batteries and supercapacitors, owing to their potential for enhancing safety and flexibility. In this work, employs a solution casting technique to prepare SPEs, utilizing chitosan‐dextran blends as the polymer matrix. Ammonium thiocyanate (NH4SCN) is incorporated as a charge carrier, while honey...