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Carboxylated styrene‐butadiene latex (XSBL), attributed to its insufficient adhesion and poor water resistance, cannot be widely popularized in the adhesive industry. Herein, a novel XSBL‐based resin with high‐strength yet water‐resistant was reported, in which the butadiene macromolecular chains were grafted with acrylonitrile (AN) and acrylic acid‐2 hydroxyethyl ester (HEA) molecules, the crosslinking...