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N‐type Mg3(Bi, Sb)2‐based thermoelectric (TE) alloys show great promise for solid‐state power generation and refrigeration, owing to their excellent figure‐of‐merit (ZT) and using cheap Mg. However, their rigorous preparation conditions and poor thermal stability limit their large‐scale applications. Here, this work develops an Mg compensating strategy to realize n‐type Mg3(Bi, Sb)2 by a facile melting‐sintering...
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