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The possibility to obtain molecular nonlinear optical switches with high on/off contrast is discussed in boronated azobenzene derivatives from a computational investigation conducted at the Density Functional Theory (DFT) level. An optimized situation is found in the case of 2-(1-phenylazo-2-naphthol)-1,3,2-benzodioxaborole in which the computed NLO response could decrease 8.5 times after E to Z isomerization...
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