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Grand canonical Monte Carlo and configurational bias Monte Carlo techniques were employed to simulate the adsorption of binary mixtures of butane isomers and quaternary mixtures in nine zeolites at 300K. For binary mixtures the results show there is a critical pore size, which is 10-membered-ring about 5.6Å. The channel sizes of BEA, ISV, MOR and CFI are larger than this critical pore size, they prefer...
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