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Chiral inorganic quasi‐2D perovskites are prepared by self‐assembling 3D perovskites in solution for the first time. The quasi‐2D perovskite synthesized is a pure‐phase perovskite with <n> = 3 and is periodically arranged, which is a big breakthrough in quasi‐2D inorganic perovskites. With the individual chiral CsPbBr3 nanocrystals (NCs) assemble into quasi‐2D perovskite, the g‐factor significantly...
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