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Macroscopic measurements show that Pb(II) uptake on iron-(hydr)oxides can be altered significantly by dissolved carbonate (enhanced up to 18% at pH 5 and decreased above pH ∼6.5 in analyses at 1 atm CO 2 ). This study elucidates the molecular-scale processes giving rise to these macroscopic effects by characterizing the structures of Pb(II) sorption complexes formed on goethite (α-FeOOH) in...
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