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A model composite is used to simulate the interphase between an allylamine/1,7‐octadiene plasma copolymer‐coated fiber and an epoxy resin. Time‐of‐flight secondary‐ion mass spectrometry (ToF‐SIMS) is used to identify the structure of the interacting polymers and the locus of failure. The crack propagates near to one of the glass surfaces where a bonded semi‐interpenetrating network forms. The effect...
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