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Desorption in the Na/Cu(111) system induced by an electronic excitation is studied using a quantal approach. The system is excited by a laser pulse in the fs range to the Na ∗ state corresponding to the transient capture of an electron by the alkali adsorbate. The present quantal approach describes on an equal footing the laser-induced vibrational excitation of the adsorbate in the adsorption...
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