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The efficiency of photolysis in the ablation of thick C 6 H 5 Cl films at 248 nm is probed over 40-300 mJ/cm 2 by means of time-of-flight quadrupole mass spectrometry. Up to 150 mJ/cm 2 , the photolysis yield is considerably smaller than that in the gas-phase. We argue that because of plume ejection well after the laser pulse, photolysis occurs exclusively in the...
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