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The first circularly polarized OLED (CP‐OLED) based on a chiral lanthanide complex is developed. With a simple architecture, this proof‐of‐concept device attains the highest polarization reported so far and additionally presents the first example of a Ln‐based OLED that can be turned into a CP‐OLED, fully retaining the special features of Ln‐based OLEDs.
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