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The infrared (IR) chemiluminescence studies of CO 2 formed during steady-state CO oxidation over Pd(111), Pt(111), and Rh(111) surfaces were carried out. Analysis of their emission spectra indicates that the order of the average vibrational temperature (TVAV) values of CO 2 formed during CO oxidation was as follows: Pd(111)>Pt(111)>Rh(111), and the order is coincident with the...
The infrared (IR) chemiluminescence spectra of CO 2 were measured during steady-state CO oxidation by O 2 , NO and N 2 O over Pd(110) surface. Kinetics of these reactions were studied using a molecular-beam reaction system, and the order of the activity was as follows: CO+O 2 >CO+NO>CO+N 2 O. From the analysis of the IR emission spectra, it is found that...
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