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A novel Ru π‐expanded terpyridyl sensitizer, referred to as HIS‐2, is prepared based on the molecular design strategy of substitution with a moderately electron‐donating 4‐methylstyryl group onto the terpyridyl ligand. The HIS‐2 dye exhibits a slightly increased metal‐to‐ligand charge transfer (MLCT) absorption at around 600 nm and an intense π–π* absorption in the UV region compared with a black...
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