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Total oxidation of toluene over a CuO–CeO2/Al2O3 catalyst was studied by means of Temporal Analysis of Products (TAP) at temperatures of 723–873K in the absence and presence of oxygen (molar toluene:oxygen ratio=1:9) at degrees of reduction of the catalyst up to 0.42. A single set of kinetic parameters corresponding to the steps of the detailed mechanism can describe the experimental data. A detailed...
Single‐event microkinetic (SEMK) modeling is applied to catalytic cracking of 2,2,4‐trimethylpentane on a series of faujasites with Si/Al ratio ranging from 2.6 to 30. Standard activation entropies of the various elementary reaction families are calculated a priori from transition state theory and statistical thermodynamics, while activation energies are estimated on a reference faujasite by regression...
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