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New pyridylthioether-based dendrons bearing a thiol moiety at their focal point have been prepared by a convergent synthetic approach. These dendrons were readily attached to a Fe 2 (CO) 6 core to generate two-directional dendritic molecules incorporating an iron-carbonyl cluster.
Unsymmetrical pyridylthioether monomers derived from 2,6-bis(hydroxymethyl)-3-hydroxypyridine hydrochloride have been used to synthesize dendritic structures by a convergent route. The coupling of the monomers has been achieved by the Mitsunobu reaction. The presence of repeating SNS pincer units makes thesemolecules precursors of metallodendrimers. The complexation of each binding site with palladium...
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