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It is reported herein that by exploiting the commonly shared bicyclic decahydroquinoline motif, a gold‐catalyzed enamide–alkyne cycloisomerization reaction is developed to access tricyclic cores in a simple way. These tricyclic cores further serve as an advanced platform for the divergent enantioselective collective total syntheses of five Lycopodium alkaloids, belonging to three different structural...
Alles im Griff: Optimierungsstudien an zweizähnigen P,N‐Liganden L offenbaren die Bedeutung einer festgelegten Konformation für das intermolekulare Abfangen reaktiver α‐Oxogoldcarben‐Zwischenstufen. Das Resultat ist eine hoch effiziente und breit anwendbare Synthese von Carboxymethylketonen aus leicht zugänglichen Carbonsäuren und endständigen Alkinen unter milden Reaktionsbedingungen.
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