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The mutual interplay between pnicogen–π and tetrel bond in the formation of PF3⊥X–Pyr…SiH3CN ternary complexes has been investigated via a computational chemistry at MP2/aug-cc-pVDZ level of theory. We proved by computational NMR data the effect of electron-withdrawing and electron-donating substituents on 1tJ(N-Si) across 15N...35Si tetrel bonds was investigated at M06-2X/aug-cc-pVDZ levels of theory...
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