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Rechargeable magnesium batteries (RMBs) are considered as one of the most promising candidates for next‐generation batteries. However, the popularization of RMBs is seriously plagued due to the lack of suitable non‐nucleophilic electrolytes and the passivation of Mg anode. Herein, a novel non‐nucleophilic electrolyte is developed by introducing (s)‐1‐methoxy‐2‐propylamine (M4) into themagnesium aluminum...
Direct photocatalytic hydrogen and oxygen evolution from water splitting is an attractive approach for producing chemical fuels. In this work, a novel fluorenone‐based covalent organic framework (COF‐SCAU‐2) is successfully exfoliated into ultrathin three‐layer nanosheets (UCOF‐SCAU‐2) for photocatalytic overall water splitting (OWS) under visible light. The ultrathin structures of UCOF‐SCAU‐2 greatly...
Covalent organic frameworks (COFs) have shown great promise for photocatalytic hydrogen evolution via water splitting. However, the four‐electron oxidation of water remains elusive toward oxygen evolution. Enabling this water oxidation pathway is critical to improve the yield and maximize atom utilization efficiency. A Z‐scheme heterojunction is proposed for overcoming fundamental issues in COF‐based...