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Hydrodeoxygenation (HDO) of phenol over nickel nano-particles of different size (5–22nm) supported on SiO2 has been investigated in a batch reactor at 275°C and 100bar. Deoxygenation was only observed as a consecutive step of initial hydrogenation of phenol at the given conditions. Both the hydrogenation and deoxygenation reaction were found to be Ni-particle size dependent. Rapid hydrogenation of...
The dehydrogenation of ethanol via acetaldehyde for the synthesis of acetic acid over a Cu based catalyst in a new process is reported. Specifically, we have studied a Cu on SiO 2 catalyst which has shown very high selectivity to acetic acid via acetaldehyde compared to competing condensation routes. The dehydrogenation experiments were carried out in a flow through lab scale tubular reactor...
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