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Although oxygen redox in Li‐rich layered cathodes can boost the available capacity over 250 mAh g−1, it also brings a rapid capacity fade upon long‐term cycling and serious safety issue during thermal abuse. To circumvent these problems, an integrated strategy via interlayer regulation at surface and the delocalization of Li2MnO3‐like domain on bulk is proposed. The controllable interlayer by atomic...
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