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The 2D asymmetric benzodithiophene (BDT) unit is used as a donor unit to construct one new polymer PBDTBDD‐Th with benzo[1,2‐c:4,5‐c′]dithiophene‐4,8‐dione (BDD) as acceptor building block. In comparison to the polymer PBDTsTh‐BDD with a side chain containing a sulfur atom, the devices based on PBDTBDD‐Th/ITIC show better performance due to the introduction of carbon atoms in the side chain, which...
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