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Many unique properties arise when the 3D stacking of layered materials is disrupted, originating nanostructures. Stabilization, and further reorganization of these individual layers into complex 3D structures, can be essential to allow these properties to persist in macroscopic systems. It is demonstrated that a simple hydrothermal process, assisted by ionic liquids (ILs), can convert bulk g‐C3N4...
Ionic liquids can promote the partial exfoliation of carbon nitride (g‐C3N4), forming 3D hydrogels, as described by Hui Xu, Pulickel M. Ajayan, and co‐workers in article number 1700653. These hydrogels essentially “freeze” the nanosheets in the delaminated state, avoiding re‐stacking. Nanostructures are successfully translated to the macroscale by constructing gas sensors, which exhibit significant...
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