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Electrosynthesis of formate via CO2 reduction (CO2ER) is of great significance for completing carbon cycle, however, low CO2 utilization efficiency caused by slow reaction kinetics greatly hinder its large‐scale application. Herein, we reported a ~50 nm‐thick SnSe2 nanosheets with enriched Se vacancies, which exhibits an excellent catalytic activity for pH‐universal formate electrosynthesis. In alkaline,...