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The initial employment of cyanato groups in higher oxidation state manganese cluster chemistry, in conjunction with the gem‐diolate form of di‐2‐pyridylketone or 2,6‐diacetylpyridine dioxime chelate ligands, has afforded structurally interesting MnII/III14 and MnII/III/IV16 clusters, respectively. In both complexes, the end‐on bridging cyanato groups show an obvious preference in binding through their...
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