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Ferroelectrics with perovskite‐like layered (PL) structure are well‐known for their high Tc and the application prospect of high‐temperature‐piezoelectric sensing. In this study, the PL‐structure Eu2Ti2O7 was prepared by 1‐step high‐pressure sintering, which show the pyrochlore structure of Eu2Ti2O7 would change into PL structure at 11 GPa, 1300°C. The PL‐structure Eu2Ti2O7 is metastable, which will...
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