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All‐inorganic CsPbI3 perovskite has emerged as an important photovoltaic material due to its high thermal stability and suitable bandgap for tandem devices. Currently, the cell performance of CsPbI3 solar cells is mainly subject to a large open‐circuit voltage (VOC) deficit. Herein, a multifunctional room‐temperature molten salt, dimethylamine acetate (DMAAc) is demonstrated, which not only directly...
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