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Systematic modification of the chelating NHC‐phosphine ligand (NHC = N‐heterocyclic carbene) in highly efficient ketone hydrogenation Mn(I) catalyst fac‐[(Ph2PCH2NHC)Mn(CO)3Br] has been performed and the catalytic activity of the resulting complexes was evaluated using acetophenone as a benchmark substrate. While the variation of phosphine and NHC moieties led to inferior results than for a parent...
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