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In the antiferromagnetic ground state, below TN ≃ 5.7 K, Ca2CoSi2O7 exhibits strong magnetoelectric coupling. For a symmetry‐consistent theoretical description of this multiferroic phase, precise knowledge of its crystal structure is a prerequisite. Here we report the results of single‐crystal neutron diffraction on Ca2CoSi2O7 at temperatures between 10 and 250 K. The low‐temperature structure at...
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