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NQR measurements were performed for the charge-transfer complexes DMTTF–QBr n Cl n−4 under ambient and hydrostatic pressures in order to understand the neutral–ionic phase transition and the quantum critical behavior. The 35 Cl NQR spectrum of DMTTF–QCl 4 showed a splitting and a shift below T c , indicating the occurrence of dimerization and charge transfer...
Neutral–ionic (NI) phase transition is a reversible switching of organic charge-transfer complexes between distinct valence states by external stimuli. This phase transformation in the low-dimensional system is demonstrated to provide a variety of novel dielectric, structural, and electronic properties. Importantly, ionization of the electron donor–acceptor pairs is usually accompanied by a ferroelectric...
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