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We report the photobiochemical production of carbon monoxide by a terminal ba3‐cytochrome c oxidase from T. thermophilus HB8. FTIR and time‐resolved step‐scan FTIR spectroscopies were combined to probe this process and also monitor the concomitant binding of the produced gas to other intact ba3 molecules forming the ba3–CO complex. The activation of this mechanism by ba3‐oxidase under visible excitation...
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