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Anchoring a homogeneous catalyst onto a heterogeneous support facilitates separation of the product from the catalyst, and catalyst‐substrate interactions can also modify reactivity. Herein we describe the synthesis of composite materials comprising carbon nitride (g‐C3N4) as the heterogeneous support and the well‐established homogeneous catalyst moiety [Cp*IrCl]+ (where Cp*=η5‐C5Me5), commonly used...
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