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We have successfully grown single crystalline Sr3-xCaxRu2O7 with the range of 2.0⩽x⩽3.0 using the floating-zone method. All compounds show orthorhombic symmetry in this substitution range, but the difference between lattice constants a and b decreases with increasing Sr concentration and becomes almost zero at x=2.0. Characteristic temperatures, which correspond to antiferromagnetic ordering and structural...
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